Reliable generation of single photons is of key importance for fundamental physical experiments and quantum protocols. The periodically poled lithium niobate (LN) waveguide has shown promise for an integrated quantum source due to its large spectral tunability and high efficiency, benefiting from the quasi-phase-matching. Here we demonstrate photon-pair sources based on an LN waveguide periodically poled by a tightly focused femtosecond laser beam. The pair coincidence rate reaches ∼8000 counts per second for average pump power of 3.2 mW (peak power is 2.9 kW). Our results prove the possibility of application of the nonlinear photonics structure fabricated by femtosecond laser to the integrated quantum source. This method can be extended to three-dimensional domain structures, which provide a potential platform for steering the spatial degree of freedom of the entangled two-photon states.

Structured optical fields embedded with polarization singularities (PSs) have attracted extensive attention due to their capability to retain topological invariance during propagation. Many advances in PS research have been made over the past 20 years in the areas of mathematical description, generation and detection technologies, propagation dynamics, and applications. However, one of the most crucial and difficult tasks continues to be manipulating PSs with multiple degrees of freedom, especially in three-dimensional (3D) tailored optical fields. We propose and demonstrate the longitudinal PS lines obtained by superimposing Bessel-like modes with orthogonal polarization states on composite vector optical fields (VOFs). The embedded PSs in the fields can be manipulated to propagate robustly along arbitrary trajectories, or to annihilate, revive, and transform each other at on-demand positions in 3D space, allowing complex PS’ topological morphology and intensity patterns to be flexibly customized. Our findings could spur further research into singular optics and help with applications such as micromanipulation, microstructure fabrication, and optical encryption.

A Hardy-like proof of quantum contextuality is a compelling way to see the conflict between quantum theory and noncontextual hidden variables (NCHVs), as the latter predict that a particular probability must be zero, while quantum theory predicts a nonzero value. For the existing Hardy-like proofs, the success probability tends to 1/2 when the number of measurement settings n goes to infinity. It means the conflict between the existing Hardy-like proof and NCHV theory is weak, which is not conducive to experimental observation. Here we advance the study of a stronger Hardy-like proof of quantum contextuality, whose success probability is always higher than the previous ones generated from a certain n-cycle graph. Furthermore, the success probability tends to 1 when n goes to infinity. We perform the experimental test of the Hardy-like proof in the simplest case of n=7 by using a four-dimensional quantum system encoded in the polarization and orbital angular momentum of single photons. The experimental result agrees with the theoretical prediction within experimental errors. In addition, by starting from our Hardy-like proof, one can establish the stronger noncontextuality inequality, for which the quantum-classical ratio is higher with the same n, which provides a new method to construct some optimal noncontextuality inequalities. Our results offer a way for optimizing and enriching exclusivity graphs, helping to explore more abundant quantum properties.

Micromachining based on femtosecond lasers usually requires accurate control of the sample movement, which may be very complex and costly. Therefore, the exploration of micromachining without sample movement is valuable. Herein, we have illustrated the manipulation of optical fields by controlling the polarization or phase to vary periodically and then realized certain focal traces by real-time loading of the computer-generated holograms (CGHs) on the spatial light modulator. The focal trace is composed of many discrete focal spots, which are generated experimentally by using the real-time dynamically controlled CGHs. With the designed focal traces, various microstructures such as an ellipse, a Chinese character “Nan”, and an irregular quadrilateral grid structure are fabricated in the z-cut LiNbO3 wafers, showing good qualities in terms of continuity and homogeneity. Our method proposes a movement free solution for micromachining samples and completely abandons the high precision stage and complex movement control, making microstructure fabrication more flexible, stable, and cheaper.

We develop a method for completely shaping optical vector beams with controllable amplitude, phase, and polarization gradients along three-dimensional freestyle trajectories. We design theoretically and demonstrate experimentally curvilinear Poincaré vector beams that exhibit high intensity gradients and accurate state of polarization prescribed along the beam trajectory.

Orbital angular momentum (OAM), as a fundamental parameter of a photon, has attracted great attention in recent years. Although various properties and applications have been developed by modulating the OAM of photons, there is rare research about the non-uniform OAM. We propose and generate a new kind of continuously tunable azimuthally non-uniform OAM for the first time, to the best of our knowledge, which is carried by a hybridly polarized vector optical field with a cylindrically symmetric intensity profile and a complex polarization singularity. We also present the perfect vector optical field carrying non-uniform OAM with a fixed radius independent of topological charges, which can propagate steadily without radial separation, solving the problem of the unsteady propagation due to the broadened OAM spectrum of the non-uniform OAM. This new kind of tunable non-uniform OAM with a cylindrical symmetric intensity profile, complex polarization singularity, and propagation stability enriches the family of OAMs and can be widely used in many regions such as optical manipulation, quantum optics, and optical communications.

Optical orbital angular momentum (OAM) is a special property of photons and has evoked research onto the light–matter interaction in both classical and quantum regimes. In classical optics, OAM is related to an optical vortex with a helical phase structure. In quantum optics, photons with a twisted or helical phase structure will carry a quantized OAM. To our knowledge, however, so far, no experiment has demonstrated the fundamental property of the OAM at the single-photon level. In this Letter, we have demonstrated the average photon trajectories of twisted photons in a double-slit interference. We have experimentally captured the double-slit interference process of twisted photons by a time-gated intensified charge-coupled device camera, which is trigged by a heralded detection. Our work provides new perspectives for understanding the micro-behaviors of twisted particles and enables new applications in imaging and sensing.

Extending the length of femtosecond laser filamentation has always been desired for practical applications. Here, we demonstrate that significant extending of a single filament in BK7 glass can be achieved by constructing phase-nested beams. The filamentation and the following energy replenishment are assembled in a single phase-nested beam. The central part of the phase-nested beam is an apertured Gaussian beam, which is focused into one focal spot to produce a short filament. In contrast, the rest of the annular part converges gradually towards the central axis to continuously replenish the energy for supporting the regeneration of filaments. The common-path generating system ensures the stability of generated filaments and easily optimizes the beam parameters to obtain the longest high-quality filament due to its flexibility. In addition, we discuss the significance of continuous replenishment for extending filaments and the potential for generating more extended filaments based on this method.

We present a highly efficient method of generating and shaping ellipse perfect vector beams (EPVBs) with a prescribed ellipse intensity profile and continuously variant linear polarization state. The scheme is based on the coaxial superposition of two orthogonally polarized ellipse laser beams of controllable phase vortex serving as the base vector components. The phase-only computer-generated hologram is specifically designed by means of a modified iteration algorithm involving a complex amplitude constraint, which is able to generate an EPVB with high diffraction efficiency in the vector optical field generator. We experimentally demonstrate that the efficiency of generating the EPVB has a notable improvement from 1.83% in the conventional complex amplitude modulation based technique to 11.1% in our method. We also discuss and demonstrate the simultaneous shaping of multiple EPVBs with independent tunable ellipticity and polarization vortex in both transversal (2D) and axial (3D) focusing structures, proving potentials in a variety of polarization-mediated applications such as trapping and transportation of particles in more complex geometric circumstances.